Comment by SturgeonsLaw

Rolling up headphone wires (or any wires) works best when you create a looped bundle and alternate between overhand and underhand. It stops it from getting twisted and tangled. When done right, you can hold one end, throw the under end, and it all unfurls neatly.

Learned this from a theatre stagehand and have been using it ever since.

https://youtube.com/watch?v=CYdu7aW_pm8